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61
Subjective

$\Delta G$ is energy available to do useful work and is thus a measure of "Free energy". Show mathematically that $\Delta G$ is a measure of free energy. Find the unit of $\Delta G$. If a reaction has positive enthalpy change and positive entropy change, under what condition will the reaction be spontaneous?

Explanation

Gibbs free energy is that thermodynamic quantity of a system, the decrease in whose value during a process is equal to the maximum possible useful work that can be obtained from the system.

Mathematically, this results may be derived as follows

The relationship between heat absorbed by a system $q$, the change in its internal energy, $\Delta U$ and the work done by the system is given by the equation of the first law of thermodynamics, therefore,

$q=\Delta U+W_{\text {expansion }}+W_{\text {non-expansion }}$ .... (i)

Under constant pressure condition, the expansion work is given by $p \Delta V$. $$ \begin{aligned} \therefore \quad q & =\Delta U+p \Delta V+W_{\text {non expansion }} \quad (\because \Delta U+p \Delta V=\Delta H) \\ & =\Delta H+W_{\text {non expansion }} \quad \ldots \text { (ii) } \end{aligned}$$

For a reversible change taking place at constant temperature,

$$\Delta S=\frac{q_{\mathrm{rev}}}{T} \text { or } q_{\mathrm{rev}}=T \Delta \mathrm{S}\quad \text{.... (iii)}$$

Substituting the value of $q$ from Eq. (iii) in Eq. (ii), we get

$$\begin{aligned} T \Delta S & =\Delta H+W_{\text {non expansion }} \\ \text{or}\quad \Delta H-T \Delta S & =-W_{\text {non-expansion }}\quad \text{... (iv)} \end{aligned}$$

For a change taking place under conditions of constant temperature and pressure,

$$\Delta G=\Delta H-T \Delta S$$

Substituting this value in equation (iv), we get

$$\Delta G=-W_{\text {non expansion }}\quad \text{... (v)}$$

Thus, free energy change can be taken as a measure of work other than the work of expansion. For most changes, the work of expansion can not be converted to other useful work, whereas the non-expansion work is convertible to useful work.

Rearranging equation (v), it may write as

$\Delta G=\Delta H-T \Delta S$

If $\Delta H=$ positive and $\Delta S=$ positive, then

$\Delta G$ will be negative i.e., process will be spontaneous only when $T \Delta S>\Delta H$ in magnitude, which will be so when temperature is high.

62
Subjective

Graphically show the total work done in an expansion when the state of an ideal gas is changed reversibly and isothermally from $\left(p_i, V_i\right)$ to $\left(p_f, V_f\right)$. With the help of a $p V$ plot compare the work done in the above case with that carried out against a constant pressure $p_f$.

Explanation

(i) Total work done in an expansion when the state of an ideal gas is changed reversibly and isothermally from $\left(p_i V_i\right)$ to $\left(p_f, V_f\right)$. Reversible work is represented by the combined areas $A B C$ and $B C V_i V_f$.

(ii) Work against constant pressure, $p_f$ is represented by the area $B C V_i V_t$. Work (i) $>$ work (ii)